Band
Title
508.0 cm-1: Fe2+-O⁻ excitation of Fe2+ & O⁻ in Ferroan Magnesite
Type
Raman scattering
Assignments summary
Assignment Symmetry Mode Specie(s) Molecule/Atom Bond Multiplicity Degeneracy Contribution Resonance
Fe2+-O⁻ excitation ligand-to-metal charge-transfer Fe2+
O⁻
no
Characteristics summary
Peak position
(cm-1)
Center position
(cm-1)
Width
(cm-1)
Shape Asymmetry factor Peak intensity
(cm-1)
Peak intensity relative Peak strength Integrated intensity
(cm-2)
Integrated intensity relative Integrated strength Temperature
(K)
Pressure
(bar)
508 ± 3 - 63 ± 6 symmetric 0.0075 vw 0.038 w 295.0 1
Label
Fe2+-O⁻ excitation
Category
electronic transition

Evaluation

Level
uncertain assignment
Evaluation
undefined
Comments
also attributed to Fe2+ excitation
# Multiplicity type Degeneracy Other band
1 no
Primary specie
Fe2+
Primary specie
O⁻

Electronic modes

Label (type)
TBD (ligand-to-metal charge-transfer)
Composition
5%
Texture
crystal in plot

Temperature

Temperature
295.0 ± 5.0 K

Pressure

Pressure
1 bar
Laser wavelength
532.0 nm
Sample orientation mode
unoriented
Method #1
various
Overlap
isolated
Peak
508 ± 3 cm-1 (fit peak)
Evaluation
validated
Quality
C
Comments
possibly slightly increases with Fe fraction
FWHM
63 ± 6 cm-1 (fwhm)
Shape
symmetric
Evaluation
validated
Quality
E
Comments
increases with Mg fraction
Method
baseline corrected peak intensity
Relative intensity
0.0075 ± 0.0035
Strength
very weak (vw)
Evaluation
validated
Quality
E
Comments
maybe slight decrease with increasing Fe content, but very dispersed values
Method
width x peak intensity
Relative intensity
0.038 ± 0.016
Strength
weak (w)
Evaluation
recommended
Quality
E
Comments
decreases with Mg fraction